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Creators/Authors contains: "Kim, Ryan"

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  1. Acoustically driven ferromagnetic resonance (ADFMR) is a platform that enables efficient generation and detection of spin waves via magnetoelastic coupling with surface acoustic waves (SAWs). While previous studies successfully achieved ADFMR in ferromagnetic metals, there are only few reports on ADFMR in magnetic insulators such as yttrium iron garnet (Y3Fe5O12, YIG) despite more favorable spin wave properties, including low damping and long coherence length. The growth of high-quality YIG films for ADFMR devices is a major challenge due to poor lattice-matching and thermal degradation of the piezoelectric substrates during film crystallization. In this work, we demonstrate ADFMR of YIG thin films on LiNbO3 (LNO) substrates. We employed a SiOx buffer layer and rapid thermal annealing for crystallization of YIG films with minimal thermal degradation of LNO substrates. Optimized ADFMR device designs and time-gating measurements were used to enhance the ADFMR signal and overcome the intrinsically low magnetoelastic coupling of YIG. YIG films have a polycrystalline structure with an in-plane easy direction due to biaxial stresses induced during cooling after crystallization. The YIG device shows clear ADFMR patterns with maximum absorption for H ≈ 160 mT parallel to SAW propagation, which is consistent with our simulation results based on existing theoretical models. These results expand possibilities for developing efficient spin wave devices with magnetic insulators. 
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  2. In this work, we demonstrate the ability to simultaneously pattern fibers and fabricate functional 2D and 3D shapes (e.g., letters, mask-like structures with nose bridges and ear loops, aprons, hoods) using a single step electrospinning process. Using 2D and 3D mesh templates, electrospun fibers were preferentially attracted to the metal protrusions relative to the voids so that the pattern of the electrospun mat mimicked the woven mesh macroscopically. On a microscopic scale, the electrostatic lensing effect decreased fiber diameter and narrowed the fiber size distribution, e.g., the coefficient of variation of the fiber diameter for sample collected on a 0.6 mm mesh was 14% compared to 55% for the sample collected on foil). Functionally, the mesh did not affect the wettability of the fiber mats. Notably, the fiber patterning increased the rigidity of the fiber mat. There was a 2-fold increase in flexural rigidity using the 0.6 mm mesh compared to the sample collected on foil. Overall, we anticipate this approach will be a versatile tool for design and fabrication of 2D and 3D patterns with potential applications in personalized wound care and surgical meshes. 
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  3. null (Ed.)
    Due to the amount of data involved in emerging deep learning and big data applications, operations related to data movement have quickly become a bottleneck. Data-centric computing (DCC), as enabled by processing-in-memory (PIM) and near-memory processing (NMP) paradigms, aims to accelerate these types of applications by moving the computation closer to the data. Over the past few years, researchers have proposed various memory architectures that enable DCC systems, such as logic layers in 3D-stacked memories or charge-sharing-based bitwise operations in dynamic random-access memory (DRAM). However, application-specific memory access patterns, power and thermal concerns, memory technology limitations, and inconsistent performance gains complicate the offloading of computation in DCC systems. Therefore, designing intelligent resource management techniques for computation offloading is vital for leveraging the potential offered by this new paradigm. In this article, we survey the major trends in managing PIM and NMP-based DCC systems and provide a review of the landscape of resource management techniques employed by system designers for such systems. Additionally, we discuss the future challenges and opportunities in DCC management. 
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  4. null (Ed.)
  5. Abstract Organic semiconductor materials have recently gained momentum due to their non‐toxicity, low cost, and sustainability. Xylindein is a remarkably photostable pigment secreted by fungi that grow on decaying wood, and its relatively strong electronic performance is enabled by π–π stacking and hydrogen‐bonding network that promote charge transport. Herein, femtosecond transient absorption spectroscopy with a near‐IR probe was used to unveil a rapid excited‐state intramolecular proton transfer reaction. Conformational motions potentially lead to a conical intersection that quenches fluorescence in the monomeric state. In concentrated solutions, nascent aggregates exhibit a faster excited state lifetime due to excimer formation, confirmed by the excimer→charge‐transfer excited‐state absorption band of the xylindein thin film, thus limiting its optoelectronic performance. Therefore, extending the xylindein sidechains with branched alkyl groups may hinder the excimer formation and improve optoelectronic properties of naturally derived materials. 
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